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Chemical composition and formation mechanisms in the cathode-electrolyte interface layer of lithium manganeseoxide batteries from reactive force field (ReaxFF) based molecular dynamics

Sahithya REDDIVARI, Christian LASTOSKIE, Ruofei WU, Junliang ZHANG

Frontiers in Energy 2017, Volume 11, Issue 3,   Pages 365-373 doi: 10.1007/s11708-017-0500-8

Abstract: Lithium manganese oxide (LiMn O ) is a principal cathode material for high power and high energy densityHowever, there are well-documented problems with capacity fade of lithium ion batteries containing LiMncell containing LiMn O ages, suggesting that active material loss by dissolution of divalent manganesefrom the LiMn O surface is the primary reason for reduced cell life in LiMn O batteries.To improve the retention of manganese in the active material, it is key to understand the reactions that

Keywords： lithium manganese oxide batteries     reactive force field (ReaxFF)     cathode-electrolyte interface layer     molecular    

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Preparation of lithium ion-sieve and utilizing in recovery of lithium from seawater

Lu WANG, Changgong MENG, Wei MA

Frontiers of Chemical Science and Engineering 2009, Volume 3, Issue 1,   Pages 65-67 doi: 10.1007/s11705-009-0105-9

Abstract: Lithium is one of the most important light metals, which is widely used as raw materials for large-capacityrechargeable batteries, light aircraft alloys and nuclear fusion fuel.resource of lithium.for Li , especially the spinel manganese oxides (SMO), which among the series of ion-sieves, has becomethe most promising adsorption material for lithium.

Keywords： lithium     ion-sieve     seawater     spinel manganese oxide    

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A review on the development of electrolytes for lithium-based batteries for low temperature applications

Frontiers in Energy 2023, Volume 17, Issue 1,   Pages 43-71 doi: 10.1007/s11708-022-0853-5

Abstract: The aerospace industry relies heavily on lithium-ion batteries in instrumentation such as satellitesdemands for greater energy storage rise, new materials also need to be adopted involving next generation lithium-ionWith these objectives in mind, tailoring of the electrolyte with higher-capacity materials such as lithiumreview paper highlights the progression of electrolyte research for low temperature performance of lithium-ionbatteries over the previous several decades.

Keywords： electrolyte     lithium-ion     low temperature     aerospace     solid-electrolyte interface    

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Recent Advances in Energy Chemical Engineering of Next-Generation Lithium Batteries Review

Xue-Qiang Zhang, Chen-Zi Zhao, Jia-Qi Huang, Qiang Zhang

Engineering 2018, Volume 4, Issue 6,   Pages 831-847 doi: 10.1016/j.eng.2018.10.008

Abstract:

Rechargeable lithium-ion batteries (LIBs) afford a profound impact on our modern daily life.Next-generation lithium (Li) batteries, which employ Li metal as the anode and intercalation or conversionThis review starts by summarizing the electrolytes for next-generation Li batteries.Key challenges and recent progress in lithium-ion, lithium–sulfur, and lithium–oxygen batteriesFinally, possible directions for further development in Li batteries are presented.

Keywords： Lithium-ion batteries     Lithium–sulfur batteries     Lithium–oxygen batteries     Lithium metal     Solid-state batteries    

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Catalytic activity of manganese oxide supported on alumina in the synthesis of quinoxalines

Rekha M., H. Kathyayini, N. Nagaraju

Frontiers of Chemical Science and Engineering 2013, Volume 7, Issue 4,   Pages 415-421 doi: 10.1007/s11705-013-1360-3

Abstract: Two catalysts, alumina and manganese oxide supported on alumina, have been prepared by calcination and

Keywords： alumina     manganese oxide deposited on alumina     quinoxaline synthesis    

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Continuous amino-functionalized University of Oslo 66 membranes as efficacious polysulfide barriers for lithium−sulfur batteries

Frontiers of Chemical Science and Engineering 2023, Volume 17, Issue 2,   Pages 194-205 doi: 10.1007/s11705-022-2206-7

Abstract: The shuttle effect of soluble polysulfides is a serious problem impeding the development of lithium−sulfurbatteries.can act as ionic sieves and serve as barriers to polysulfides transport while allowing the passage of lithiumTherefore, lithium−sulfur batteries with this interlayer show a desirable initial capacity of 999.21

Keywords： lithium−sulfur batteries     amino-functionalized University of Oslo 66 membrane     polysulfide     interlayer    

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Spent rechargeable lithium batteries in e-waste: composition and its implications

Xianlai ZENG,Jinhui LI

Frontiers of Environmental Science & Engineering 2014, Volume 8, Issue 5,   Pages 792-796 doi: 10.1007/s11783-014-0705-6

Abstract: The amount of spent rechargeable lithium batteries (RLBs) is growing rapidly owing to wide applicationof these batteries in portable electronic devices and electric vehicles, which obliges that spent RLBs

Keywords： rechargeable lithium batteries     e-waste     physical components     difference analysis     recycling    

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Localized high-concentration electrolytes for lithium metal batteries: progress and prospect

Frontiers of Chemical Science and Engineering 2023, Volume 17, Issue 10,   Pages 1354-1371 doi: 10.1007/s11705-022-2286-4

Abstract: the increasing development of digital devices and electric vehicles, high energy-density rechargeable batteriesmetal batteries due to the inevitable growth of lithium dendrites and poor interface stability.metal batteries.metal batteries are discussed.metal batteries.

Keywords： high-concentration electrolyte     localized high-concentration electrolyte     lithium metal battery     solid    

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Interlayer-confined two-dimensional manganese oxide-carbon nanotube catalytic ozonation membrane for

Frontiers of Chemical Science and Engineering 2022, Volume 16, Issue 5,   Pages 731-744 doi: 10.1007/s11705-021-2110-6

Abstract: Catalytic ozonation technology has attracted copious attention in water purification owing to its favorable oxidative degradation of pollutants and mitigation of membrane fouling capacity. However, its extensive industrial application has been restricted by the low ozone utilization and limited mass transfer of the short-lived radical species. Interlayer space-confined catalysis has been theoretically proven to be a viable strategy for achieving high catalytic efficiency. Here, a two-dimensional MnO2-incorporated ceramic membrane with tunable interspacing, which was obtained via the intercalation of a carbon nanotube, was designed as a catalytic ozonation membrane reactor for degrading methylene blue. Benefiting from the abundant catalytic active sites on the surface of two-dimensional MnO2 as well as the ultralow mass transfer resistance of fluids due to the nanolayer confinement, an excellent mineralization effect, i.e., 1.2 mg O3(aq) mg–1 TOC removal (a total organic carbon removal rate of 71.5%), was achieved within a hydraulic retention time of 0.045 s of pollutant degradation. Further, the effects of hydraulic retention time and interlayer spacing on methylene blue removal were investigated. Moreover, the mechanism of the catalytic ozonation employing catalytic ozonation membrane was proposed based on the contribution of the Mn(III/IV) redox pair to electron transfer to generate the reactive oxygen species. This innovative two-dimensional confinement catalytic ozonation membrane could act as a nanoreactor and separator to efficiently oxidize organic pollutants and enhance the control of membrane fouling during water purification.

Keywords： catalytic membrane reactor     catalytic ozonation     nanoconfinement     two-dimensional manganese oxide    

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Two-phase early prediction method for remaining useful life of lithium-ion batteries based on a neural

Frontiers in Energy doi: 10.1007/s11708-023-0906-4

Abstract: Lithium-ion batteries (LIBs) are widely used in transportation, energy storage, and other fields.The prediction of the remaining useful life (RUL) of lithium batteries not only provides a referenceBy testing four batteries under different working conditions, the RMSE of all capacity estimation is

Keywords： lithium-ion batteries     RUL prediction     double exponential model     neural network     Gaussian process regression    

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zirconium-based metal-organic framework-801 films on carbon cloth as shuttle-inhibiting interlayers for lithium-sulfurbatteries

Frontiers of Chemical Science and Engineering 2022, Volume 16, Issue 4,   Pages 511-522 doi: 10.1007/s11705-021-2068-4

Abstract: Lithium-sulfur batteries have been regarded as the next-generation rechargeable batteries due to theirNevertheless, the shuttle effect of lithium polysulfides has hindered the development of lithium-sulfurbatteries.batteries.Based on the above advantages, the lithium-sulfur battery, with the proposed interlayer, delivers an

Keywords： lithium-sulfur batteries     metal-organic framework-801 film     interlayer     shuttle effect    

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Promoting Si-graphite composite anodes with SWCNT additives for half and NCM811 full lithium ion batteries

Jingning SHAN, Xiaofang YANG, Chao YAN, Yiguang JU, Lin CHEN, Fang ZHAO

Frontiers in Energy 2019, Volume 13, Issue 4,   Pages 626-635 doi: 10.1007/s11708-019-0650-y

Abstract: Single wall carbon nanotube (SWCNT) additives were formulated into µm-Si-graphite composite electrodes and tested in both half cells and full cells with high nickel cathodes. The critical role of small amount of SWCNT addition (0.2 wt%) was found for significantly improving delithiation capacity, first cycle coulombic efficiency (FCE), and capacity retention. Particularly, Si (10 wt%)-graphite electrode exhibits 560 mAh/g delithiation capacity and 92% FCE at 0.2 C during the first charge-discharge cycle, and 91% capacity retention after 50 cycles (0.5 C) in a half cell. Scanning electron microscope (SEM) was used to illustrate the electrode morphology, compositions and promoting function of the SWCNT additives. In addition, full cells assembled with high nickel-NCM811 cathodes and µm-Si-graphite composite anodes were evaluated for the consistence between half and full cell performance, and the consideration for potential commercial application. Finally, criteria to assess Si-containing anodes are proposed and discussed from an industrial perspective.

Keywords： lithium-ion battery     Si anode     Si-graphite composite     single wall carbon nanotube (SWCNT)     NCM811    

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Multi-effect anthraquinone-based polyimide enclosed SnO/reduced graphene oxide composite as high-performanceanode for lithium-ion battery

Frontiers of Chemical Science and Engineering 2023, Volume 17, Issue 9,   Pages 1231-1243 doi: 10.1007/s11705-023-2306-z

Abstract: The cycling stability of SnO2 anode as lithium-ion battery is poor due to volume expansionHerein, the SnO2 enclosed with anthraquinone-based polyimide/reduced graphene oxide compositeIn addition, the introduction of reduced graphene oxide cannot only improve the stability of polyimidethe multiple effects of anthraquinone-based polyimide and the synergistic effect of reducing graphene oxide

Keywords： anthraquinone-based polyimide     multi-effect     tin dioxide     reduced graphene oxide     lithium-ion battery    

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Ion conduction path in composite solid electrolytes for lithium metal batteries: from polymer rich to

Zhouyu ZHANG, Hao CHEN, Zhenglin HU, Shoubin ZHOU, Lan ZHANG, Jiayan LUO

Frontiers in Energy 2022, Volume 16, Issue 5,   Pages 706-733 doi: 10.1007/s11708-022-0833-9

Abstract: Solid-state electrolytes (SSEs) can address the safety issue of organic electrolyte in rechargeable lithiumbatteries.and brittle but more conducting ceramics can take advantage of the individual system for solid-state lithiummetal batteries (SSLMBs).

Keywords： composite solid electrolytes     active filler/framework     ion conduction path     interphase compatibility     multilayer design    

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Fabrication of layered structure VS anchor in 3D graphene aerogels as a new cathode material for lithiumion batteries

Frontiers in Energy 2019, Volume 13, Issue 3,   Pages 597-602 doi: doi:10.1007/s11708-018-0576-9

Abstract: more and more attention for its high theoretical capacity (449 mAh/g with 3e− transfer) in lithiumion batteries (LIBs).

Keywords： VS4     graphene aerogels     cathode     lithium storage    

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Title Author Date Type Operation

Chemical composition and formation mechanisms in the cathode-electrolyte interface layer of lithium manganeseoxide batteries from reactive force field (ReaxFF) based molecular dynamics

Sahithya REDDIVARI, Christian LASTOSKIE, Ruofei WU, Junliang ZHANG

Journal Article

Preparation of lithium ion-sieve and utilizing in recovery of lithium from seawater

Lu WANG, Changgong MENG, Wei MA

Journal Article

A review on the development of electrolytes for lithium-based batteries for low temperature applications

Journal Article

Recent Advances in Energy Chemical Engineering of Next-Generation Lithium Batteries

Xue-Qiang Zhang, Chen-Zi Zhao, Jia-Qi Huang, Qiang Zhang

Journal Article

Catalytic activity of manganese oxide supported on alumina in the synthesis of quinoxalines

Rekha M., H. Kathyayini, N. Nagaraju

Journal Article

Continuous amino-functionalized University of Oslo 66 membranes as efficacious polysulfide barriers for lithium−sulfur batteries

Journal Article

Spent rechargeable lithium batteries in e-waste: composition and its implications

Xianlai ZENG,Jinhui LI

Journal Article

Localized high-concentration electrolytes for lithium metal batteries: progress and prospect

Journal Article

Interlayer-confined two-dimensional manganese oxide-carbon nanotube catalytic ozonation membrane for

Journal Article

Two-phase early prediction method for remaining useful life of lithium-ion batteries based on a neural

Journal Article

zirconium-based metal-organic framework-801 films on carbon cloth as shuttle-inhibiting interlayers for lithium-sulfurbatteries

Journal Article

Promoting Si-graphite composite anodes with SWCNT additives for half and NCM811 full lithium ion batteries

Jingning SHAN, Xiaofang YANG, Chao YAN, Yiguang JU, Lin CHEN, Fang ZHAO

Journal Article

Multi-effect anthraquinone-based polyimide enclosed SnO/reduced graphene oxide composite as high-performanceanode for lithium-ion battery

Journal Article

Ion conduction path in composite solid electrolytes for lithium metal batteries: from polymer rich to

Zhouyu ZHANG, Hao CHEN, Zhenglin HU, Shoubin ZHOU, Lan ZHANG, Jiayan LUO

Journal Article

Fabrication of layered structure VS anchor in 3D graphene aerogels as a new cathode material for lithiumion batteries

Journal Article